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Nanostructured ZnO as a structural template for the growth of ZIF-8 with tunable hierarchical porosity for CO2 conversion

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Abstract

We report a new approach to introduce hierarchical porosity into ZIF-8 by using three-dimensional nanostructured porous ZnO as a structural template. Importantly, the textural properties of these nanostructures can be tuned simply by varying the size of the polymeric templates used for the preparation of ZnO. Moreover, the growth of ZIF-8 crystals on ZnO and the resulting hierarchical porosity enabled enhanced catalytic activity for the conversion of CO2 into cyclic carbonates through an atom economy reaction in high yields with exceptional product selectivity.

Graphical abstract: Nanostructured ZnO as a structural template for the growth of ZIF-8 with tunable hierarchical porosity for CO2 conversion

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Publication details

The article was received on 12 Dec 2016, accepted on 23 Jan 2017 and first published on 24 Jan 2017


Article type: Communication
DOI: 10.1039/C6CE02549H
Citation: CrystEngComm, 2017, Advance Article
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    Nanostructured ZnO as a structural template for the growth of ZIF-8 with tunable hierarchical porosity for CO2 conversion

    M. Kim, D. Kim, J. Y. Seo, O. Buyukcakir and A. Coskun, CrystEngComm, 2017, Advance Article , DOI: 10.1039/C6CE02549H

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