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Formal arylation of NH3 to produce diphenylamines over supported Pd catalysts

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Abstract

In the presence of supported Pd nanoparticle catalysts, e.g., Pd/Al2O3, various diphenylamines could be synthesized through acceptorless formal arylation using NH3 or its surrogates, e.g., urea, as nitrogen sources and cyclohexanones as arylation sources. The observed catalysis was truly heterogeneous, and the catalyst was reusable with retention of its high catalytic performance.

Graphical abstract: Formal arylation of NH3 to produce diphenylamines over supported Pd catalysts

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Publication details

The article was received on 28 Aug 2017, accepted on 11 Sep 2017 and first published on 11 Sep 2017


Article type: Communication
DOI: 10.1039/C7CC06737B
Citation: Chem. Commun., 2017, Advance Article
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    Formal arylation of NH3 to produce diphenylamines over supported Pd catalysts

    Y. Koizumi, K. Taniguchi, X. Jin, K. Yamaguchi, K. Nozaki and N. Mizuno, Chem. Commun., 2017, Advance Article , DOI: 10.1039/C7CC06737B

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