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Issue 64, 2017
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Oxidation-induced C–H amination leads to a new avenue to build C–N bonds

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Abstract

In this work, we develop an oxidation-induced C–H functionalization strategy, which not only leads to a new avenue to build C–N bonds, but also leads to different site-selectivity compared with “classic directing-groups”. The high selectivity of our new catalytic system originates from the heterogeneous electron-density distribution of the radical cation species which are induced by single electron transfer between the aromatics and oxidant-Cu(II) species.

Graphical abstract: Oxidation-induced C–H amination leads to a new avenue to build C–N bonds

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Publication details

The article was received on 27 Jun 2017, accepted on 13 Jul 2017 and first published on 13 Jul 2017


Article type: Communication
DOI: 10.1039/C7CC04955B
Citation: Chem. Commun., 2017,53, 8984-8987
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    Oxidation-induced C–H amination leads to a new avenue to build C–N bonds

    H. Yi, Z. Tang, C. Bian, H. Chen, X. Qi, X. Yue, Y. Lan, J. Lee and A. Lei, Chem. Commun., 2017, 53, 8984
    DOI: 10.1039/C7CC04955B

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