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Tracking thermal-induced amorphization of a zeolitic imidazolate framework via synchrotron in situ far-infrared spectroscopy

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Abstract

We present the first use of in situ far-infrared spectroscopy to analyze the thermal amorphization of a zeolitic imidazolate framework material. We explain the nature of vibrational motion changes during the amorphization process and reveal new insights into the effect that temperature has on the Zn–N tetrahedra.

Graphical abstract: Tracking thermal-induced amorphization of a zeolitic imidazolate framework via synchrotron in situ far-infrared spectroscopy

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Publication details

The article was received on 15 Mar 2017, accepted on 06 Jun 2017 and first published on 06 Jun 2017


Article type: Communication
DOI: 10.1039/C7CC01985H
Citation: Chem. Commun., 2017, Advance Article
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    Tracking thermal-induced amorphization of a zeolitic imidazolate framework via synchrotron in situ far-infrared spectroscopy

    M. R. Ryder, T. D. Bennett, C. S. Kelley, M. D. Frogley, G. Cinque and J. Tan, Chem. Commun., 2017, Advance Article , DOI: 10.1039/C7CC01985H

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