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Issue 25, 2017
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Isotopically enriched polymorphs of dysprosium single molecule magnets

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Abstract

A triclinic polymorph Dy(t) and a monoclinic polymorph Dy(m) of [Dy(tta)3(L)] with L = 4-[6-(1,3-benzothiazol-2-yl)pyridin-3-yl]-4′,5′-bis(methylthio)tetrathiafulvene behave as Single-Molecule Magnets with hysteresis loops opened at zero field. Magnetic properties were enhanced through magnetic dilution and 164Dy isotopic enrichment which definitively support the importance of isotopes for the control of quantum magnets.

Graphical abstract: Isotopically enriched polymorphs of dysprosium single molecule magnets

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Publication details

The article was received on 13 Jan 2017, accepted on 06 Mar 2017 and first published on 07 Mar 2017


Article type: Communication
DOI: 10.1039/C7CC00317J
Citation: Chem. Commun., 2017,53, 3575-3578
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    Isotopically enriched polymorphs of dysprosium single molecule magnets

    Y. Kishi, F. Pointillart, B. Lefeuvre, F. Riobé, B. Le Guennic, S. Golhen, O. Cador, O. Maury, H. Fujiwara and L. Ouahab, Chem. Commun., 2017, 53, 3575
    DOI: 10.1039/C7CC00317J

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