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Volume 194, 2016
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Stimulated X-ray Raman scattering – a critical assessment of the building block of nonlinear X-ray spectroscopy

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Abstract

With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets.

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Publication details

The article was received on 29 Apr 2016, accepted on 13 Jun 2016 and first published on 14 Jun 2016


Article type: Paper
DOI: 10.1039/C6FD00103C
Citation: Faraday Discuss., 2016,194, 305-324
  • Open access: Creative Commons BY-NC license
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    Stimulated X-ray Raman scattering – a critical assessment of the building block of nonlinear X-ray spectroscopy

    V. Kimberg, A. Sanchez-Gonzalez, L. Mercadier, C. Weninger, A. Lutman, D. Ratner, R. Coffee, M. Bucher, M. Mucke, M. Agåker, C. Såthe, C. Bostedt, J. Nordgren, J. E. Rubensson and N. Rohringer, Faraday Discuss., 2016, 194, 305
    DOI: 10.1039/C6FD00103C

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