Issue 24, 2016

Slow and long-ranged dynamical heterogeneities in dissipative fluids

Abstract

A two-dimensional bidisperse granular fluid is shown to exhibit pronounced long-ranged dynamical heterogeneities as dynamical arrest is approached. Here we focus on the most direct approach to study these heterogeneities: we identify clusters of slow particles and determine their size, Nc, and their radius of gyration, RG. We show that Image ID:c6sm00784h-t1.gif, providing direct evidence that the most immobile particles arrange in fractal objects with a fractal dimension, df, that is observed to increase with packing fraction ϕ. The cluster size distribution obeys scaling, approaching an algebraic decay in the limit of structural arrest, i.e., ϕϕc. Alternatively, dynamical heterogeneities are analyzed via the four-point structure factor S4(q,t) and the dynamical susceptibility χ4(t). S4(q,t) is shown to obey scaling in the full range of packing fractions, 0.6 ≤ ϕ ≤ 0.805, and to become increasingly long-ranged as ϕϕc. Finite size scaling of χ4(t) provides a consistency check for the previously analyzed divergences of χ4(t) ∝ (ϕϕc)γχ and the correlation length ξ ∝ (ϕϕc)γξ. We check the robustness of our results with respect to our definition of mobility. The divergences and the scaling for ϕϕc suggest a non-equilibrium glass transition which seems qualitatively independent of the coefficient of restitution.

Graphical abstract: Slow and long-ranged dynamical heterogeneities in dissipative fluids

Article information

Article type
Paper
Submitted
31 Mar 2016
Accepted
17 May 2016
First published
17 May 2016

Soft Matter, 2016,12, 5461-5474

Author version available

Slow and long-ranged dynamical heterogeneities in dissipative fluids

K. E. Avila, H. E. Castillo, K. Vollmayr-Lee and A. Zippelius, Soft Matter, 2016, 12, 5461 DOI: 10.1039/C6SM00784H

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