AgPd@Pd/TiO2 nanocatalyst synthesis by microwave heating in aqueous solution for efficient hydrogen production from formic acid

Masashi Hattori; Daisuke Shimamoto; Hiroki Ago; Masaharu Tsuji

doi:10.1039/C5TA01434D

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AgPd@Pd/TiO₂ nanocatalyst synthesis by microwave heating in aqueous solution for efficient hydrogen production from formic acid†

Masashi Hattori,^a Daisuke Shimamoto,^b Hiroki Ago^a and Masaharu Tsuji*^a

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* Corresponding authors

^a Institute for Materials Chemistry and Engineering, Kyushu University, Kasuga 816-8580, Japan
E-mail: tsuji@cm.kyushu-u.ac.jp

^b Department of Applied Science for Electronics and Materials, Graduate School of Engineering Sciences, Kyushu University, Kasuga 816-8580, Japan

Abstract

Ag_100−xPd_x/TiO₂ (x = 7, 10, and 15) catalysts for hydrogen production from formic acid were synthesized in aqueous solution using MW heating. The hydrogen production rate of Ag_100−xPd_x@Pd/TiO₂ increased concomitantly with decreasing x. The best catalytic activity ever reported was obtained for Ag₉₃Pd₇@Pd/TiO₂ among all heterogeneous catalysts.

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Article information

DOI: https://doi.org/10.1039/C5TA01434D
Article type: Communication
Submitted: 24 Feb 2015
Accepted: 14 Apr 2015
First published: 15 Apr 2015

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J. Mater. Chem. A, 2015,3, 10666-10670

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AgPd@Pd/TiO₂ nanocatalyst synthesis by microwave heating in aqueous solution for efficient hydrogen production from formic acid

M. Hattori, D. Shimamoto, H. Ago and M. Tsuji, J. Mater. Chem. A, 2015, 3, 10666 DOI: 10.1039/C5TA01434D

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Journal of Materials Chemistry A