Issue 17, 2014

NIR-Selective electrochromic heteromaterial frameworks: a platform to understand mesoscale transport phenomena in solid-state electrochemical devices

Abstract

We report here the first solid-state, NIR-selective electrochromic devices. Critical to device performance is the arrangement of nanocrystal-derived electrodes into heteromaterial frameworks, where hierarchically porous ITO nanocrystal active layers are infiltrated by an ion-conducting polymer electrolyte with mesoscale periodicity. Enhanced coloration efficiency and transport are realized over unarchitectured electrodes in devices, paving the way towards new smart windows technologies.

Graphical abstract: NIR-Selective electrochromic heteromaterial frameworks: a platform to understand mesoscale transport phenomena in solid-state electrochemical devices

Supplementary files

Article information

Article type
Paper
Submitted
14 Nov 2013
Accepted
08 Jan 2014
First published
08 Jan 2014

J. Mater. Chem. C, 2014,2, 3328-3335

NIR-Selective electrochromic heteromaterial frameworks: a platform to understand mesoscale transport phenomena in solid-state electrochemical devices

T. E. Williams, C. M. Chang, E. L. Rosen, G. Garcia, E. L. Runnerstrom, B. L. Williams, B. Koo, R. Buonsanti, D. J. Milliron and B. A. Helms, J. Mater. Chem. C, 2014, 2, 3328 DOI: 10.1039/C3TC32247E

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