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Issue 24, 2013
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Visible-light-induced WO3/g-C3N4 composites with enhanced photocatalytic activity

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Abstract

Novel WO3/g-C3N4 composite photocatalysts were prepared by a calcination process with different mass contents of WO3. The photocatalysts were characterized by thermogravimetric analysis (TG), powder X-ray diffraction (XRD), scanning electron microscopy (SEM) and energy dispersive X-ray spectrometry (EDS), high-resolution transmission electron microscopy (HRTEM), UV-vis diffuse reflection spectroscopy (DRS), X-ray photoelectron spectroscopy (XPS), photoluminescence (PL) and electrochemical impedance spectroscopy (EIS). The photocatalytic activity of the photocatalysts was evaluated by degradation of methylene blue (MB) dye and 4-chlorophenol (4-CP) under visible light. The results indicated that the WO3/g-C3N4 composite photocatalysts showed higher photocatalytic activity than both the pure WO3 and pure g-C3N4. The optimum photocatalytic activity of WO3/g-C3N4 at a WO3 mass content of 9.7% under visible light irradiation was up to 4.2 times and 2.9 times as high as that of the pure WO3 and pure g-C3N4, respectively. The remarkably increased performance of WO3/g-C3N4 was mainly attributed to the synergistic effect between the interface of WO3 and g-C3N4, including enhanced optical absorption in the visible region, enlarged specific surface areas and the suitable band positions of WO3/g-C3N4 composites.

Graphical abstract: Visible-light-induced WO3/g-C3N4 composites with enhanced photocatalytic activity

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Publication details

The article was received on 12 Jan 2013, accepted on 03 Apr 2013 and first published on 04 Apr 2013


Article type: Paper
DOI: 10.1039/C3DT00115F
Citation: Dalton Trans., 2013,42, 8606-8616
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    Visible-light-induced WO3/g-C3N4 composites with enhanced photocatalytic activity

    L. Huang, H. Xu, Y. Li, H. Li, X. Cheng, J. Xia, Y. Xu and G. Cai, Dalton Trans., 2013, 42, 8606
    DOI: 10.1039/C3DT00115F

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