Chelating alkylidene ligands as pacifiers for ruthenium catalysed olefin metathesis

Yuval Vidavsky; Aviel Anaby; N. Gabriel Lemcoff

doi:10.1039/C1DT11404B

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Dalton Transactions

Issue 1, 2012

The international journal for inorganic, organometallic and bioinorganic chemistry

Impact Factor 3.838 48 Issues per Year Indexed in MEDLINE

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Chelating alkylidene ligands as pacifiers for ruthenium catalysed olefin metathesis

Yuval Vidavsky,^a Aviel Anaby^a and N. Gabriel Lemcoff*^a

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Chemistry Ben-Gurion University of the Negev Beer-Sheva, Israel
E-mail: lemcoff@bgu.ac.il

Dalton Trans., 2012,41, 32-43

DOI: 10.1039/C1DT11404B
Received 25 Jul 2011, Accepted 12 Sep 2011
First published online 24 Oct 2011

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Abstract
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Olefin metathesis catalysed by ruthenium has emerged at the frontier of modern synthetic chemistry. The desire to enhance catalyst stability, gain control over the catalytic process and deepen the understanding of the mechanisms of metathesis has yielded a class of latent ruthenium precatalysts of delayed initiation and with switchable activity. One of the main methodologies developed for this purpose has been the introduction of tethered carbene ligands. Herein we track the evolution of ruthenium based metathesis catalysts bearing chelated alkylidenes, from the early oxygen Hoveyda type benzylidenes to the latent sulphur containing complexes.

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