The first 3d-4f clusters built using derivatised salicylaldoximes (R-saoH2) describe unusual hexagonal prisms. Replacement of the paramagnetic Gd(III) ions with diamagnetic Ln(III) ions allows for a more thorough understanding of the magnetic properties, whilst replacement with Tb(III) doubles Ueff.
![Graphical abstract: Enhancing Ueff in oxime-bridged [MnIII6LnIII2] hexagonal prisms](/en/Image/Get?imageInfo.ImageType=GA&imageInfo.ImageIdentifier.ManuscriptID=C1DT10154D&imageInfo.ImageIdentifier.Year=2011)
G. Rigaux, R. Inglis, S. Morrison, A. Prescimone, C. Cadiou, M. Evangelisti and E. K. Brechin, Dalton Trans., 2011, 40, 4797 DOI: 10.1039/C1DT10154D
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