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Issue 28, 2011
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Tunable single-site ruthenium catalysts for efficient water oxidation

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Abstract

The catalyticwater oxidation activity of mononuclear ruthenium complexes comprising a pyridine-functionalized abnormal triazolylidene ligand can be adjusted by modification of the triazolylidene substituents, which is readily achieved through click-type cycloaddition chemistry, affording some of the most active ruthenium catalysts known thus far for water oxidation (TONs > 400, TOFs close to 7000 h−1).

Graphical abstract: Tunable single-site ruthenium catalysts for efficient water oxidation

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Publication details

The article was received on 04 May 2011, accepted on 01 Jun 2011 and first published on 16 Jun 2011


Article type: Communication
DOI: 10.1039/C1CC12615F
Citation: Chem. Commun., 2011,47, 8058-8060
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    Tunable single-site ruthenium catalysts for efficient water oxidation

    L. Bernet, R. Lalrempuia, W. Ghattas, H. Mueller-Bunz, L. Vigara, A. Llobet and M. Albrecht, Chem. Commun., 2011, 47, 8058
    DOI: 10.1039/C1CC12615F

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