The onset of molecular condensation: hydrogen

J. H. Morilla; J. M. Fernández; G. Tejeda; S. Montero

doi:10.1039/C003376F

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Physical Chemistry Chemical Physics

Issue 38, 2010

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The onset of molecular condensation: hydrogen

J. H. Morilla , J. M. Fernández , G. Tejeda and S. Montero

Phys. Chem. Chem. Phys., 2010,12, 12060-12064

DOI: 10.1039/C003376F
Received 18 Feb 2010, Accepted 18 May 2010
First published on the web 03 Aug 2010

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Abstract
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The very first steps of condensation as studied experimentally in the simplest molecular system (para-H₂) are reported. The fast time–space evolution of the nascent clusters have been measured using state-of-the-art Raman spectroscopy implemented on cryogenic supersonic jets. The time-dependent onset of condensation is presented in a non-equilibrium pressure-temperature phase diagram. Dimer and trimer formation are found to obey three-body processes whose rates have been determined.

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