On the theory of intramolecular energy transfer

Rudolph A. Marcus

doi:10.1039/DC9837500103

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Faraday Discussions of the Chemical Society

Issue 0, 1983

Faraday Discussions of the Chemical Society was published from 1972 - 1991. In 1992 it continued as Faraday Discussions.

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On the theory of intramolecular energy transfer

Rudolph A. Marcus

Faraday Discuss. Chem. Soc., 1983,75, 103-115

DOI: 10.1039/DC9837500103

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Abstract
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We consider the distinguishing features of two main types of classical anharmonic motion in molecules, their quantum parallels, and conditions that classical chaos also be sufficient for “quantum chaos”. Implications are considered for experimental reaction rates, R.R.K.M. theory, spectra and a possible type of system for intramolecular laser-selective chemistry. A theory of intramolecular energy transfer between two ligands of a heavy atom is described for a system which may contain many coordinates. It is partly statistical and, for the modes of each ligand which communicate through the heavy atom, dynamical.

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On the theory of intramolecular energy transfer

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