Density functional theory investigations reveal that the intramolecular additions of N–CN bonds to alkenes proceed in a novel asynchronous and concerted mechanism, while the intramolecular addition of O–CN bonds to alkenes may occur by both concerted and stepwise pathways.
J. Zhao, G. Wang and S. Li, Chem. Commun., 2015, 51, 15450 DOI: 10.1039/C5CC06808H
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