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Chemical Science

For findings of exceptional significance from across the chemical sciences
All articles free to read, free to publish* from 2015
*Article processing charges waived for articles published in 2015 and 2016
Impact Factor 8.601 12 Issues per Year Immediacy Index 3.07
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Christine A Caputo, Lidong Wang, Radim Beranek and Erwin Reisner
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC02017D, Edge Article
A system consisting of a [NiFeSe]-hydrogenase (H2ase) grafted on the surface of a TiO2 nanoparticle modified with polyheptazine carbon nitride polymer, melon (CNx) is reported. This semi biological assembly shows...
Ahsan R Akram, Nicolaos Avlonitis, Annamaria Lilienkampf, Ana M Perez-Lopez, Neil McDonald, Sunay V Chankeshwara, Emma Scholefield, Chris Haslett, Mark Bradley and Kevin Dhaliwal
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC00960J, Edge Article
The in situ immediate detection of the presence of bacteria in the distal human lung is of significant clinical utility. Herein we describe the development and optimization of a bacterial...
Kenji Sumida, Nirmalya Moitra, Julien Reboul, Shotaro Fukumoto, Kazuki Nakanishi, Kazuyoshi Kanamori, Shuhei Furukawa and Susumu Kitagawa
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC02034D, Edge Article
The coordination replication technique is employed for the direct conversion of a macro- and mesoporous Cu(OH)2-polyacrylamide composite to three-dimensional superstructures consisting of the flexible porous coordination polymers, Cu2(bdc)2(MeOH)2 and Cu2(bdc)2(bpy)...
Volker L Deringer, Ralf P Stoffel, Matthias Wuttig and Richard Dronskowski
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC00825E, Edge Article
Antimony selenide (antimonselite, Sb2Se3) is a versatile functional material with emerging applications in solar cells. It also provides an intriguing prototype to study different modes of bonding in solid chalcogenides,...
Benjamin Lasorne, Arnaud Fihey, David Mendive-Tapia and Denis Jacquemin
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC01960E, Edge Article
Going from photochromic compounds presenting a single switchable function to multi-addressable photochromic multimers remains an extremely difficult task notably because the interactions of several photochromic units through a linker generally...
Angel M Martínez, Javier Echavarren, Ines Alonso, Nuria Rodriguez, Ramon Gomez Arrayas and Juan Carlos Carretero
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC01885D, Edge Article
The ability to establish switchable site-selectivity through catalyst control in the direct functionalization of molecules that contain distinct C-H bonds remains a demanding challenge as it would enable the construction...
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01635E, Edge Article
CTAB (cetyltrimethylammonium bromide) micelles are detected directly via the novel electrochemical method of ‘nano-impacts’ through oxidation of its bromide content.
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01977J, Edge Article
The first strategy that provides reverse-prenylated indole alkaloids that bear a characteristic bicyclo[2.2.2]diazaoctane as well as those that lack this structural motif is reported.
Steven Daly, Alexander Kulesza, Frederic Poussigue, Anne-Laure Simon, Chang Min Choi, Geoffrey Knight, Fabien Chirot, Luke MacAleese, Rodolphe Antoine and Philippe Dugourd
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01463H, Edge Article
The gas phase conformations of two amyloid beta mutants are studied by multiple techniques to elucidate the origin of the different aggregation behaviour.
Matthew D. Jones, Lauren Brady, Paul McKeown, Antoine Buchard, Pascal M. Schäfer, Lynne H. Thomas, Mary F. Mahon, Timothy J. Woodman and John P. Lowe
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01819F, Edge Article
A series complexes based on 2,2′-bipyrrolidine based salan ligands have been prepared and either isotactic or heterotactic PLA have been prepared.
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01505G, Edge Article
Natural and modified substrates coupled with LC-MS/MS analysis of products revealed the stereospecificity and stereoselectivity of a polyketide didomain.
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01227A, Perspective
This review describes recent progress on mechanistic understanding of heterogeneous catalytic dehydrogenation reactions of light alkanes.
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01772F, Edge Article
A ligand-enabled Ir-catalyzed diastereoselective and enantioselective allylic alkylation of 3-substituted indoles is reported, providing indoline products containing three contiguous stereocenters in one step with high site-, regio-, diastereo- and enantioselectivities from a wide range of readily available starting materials.
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC01482D, Edge Article
An efficient synthesis of dihydro-isoquinolines via Pd–catalyzed double C–H bonds [a C(sp2)–H and a C(sp3)–H bond] activation/annulation (CHAA) reaction is presented. During the reaction not only the two non-activated C–H...
Chun Y. Chow, Hélène Bolvin, Victoria E. Campbell, Régis Guillot, Jeff W. Kampf, Wolfgang Wernsdorfer, Frédéric Gendron, Jochen Autschbach, Vincent L. Pecoraro and Talal Mallah
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC90037A, Correction
D. L. Crossley, I. A. Cade, E. R. Clark, A. Escande, M. J. Humphries, S. M. King, I. Vitorica-Yrezabal, M. J. Ingleson and M. L. Turner
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01800E, Edge Article
Electrophilic borylation using BCl3 and benzothiadiazole to direct the C–H functionalisation of an adjacent aromatic unit produces fused boracyclic materials with minimally changed HOMO energies but significantly reduced LUMO energies.
David Y. Song, Arturo A. Pizano, Patrick G. Holder, JoAnne Stubbe and Daniel G. Nocera
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01125F, Edge Article
Proton-coupled electron transfer (PCET) is a fundamental mechanism important in a wide range of biological processes including the universal reaction catalysed by ribonucleotide reductases (RNRs) in making de novo, the building blocks required for DNA replication and repair.
Regan James Anderson, Benjamin James Compton, Ching-wen Tang, Astrid Authier-Hall, Colin Malcolm Hayman, Renata Kowalczyk, Gene William Swinerd, Paul Harris, Margaret A Brimble, David S Larsen, Olivier Gasser, Robert Weinkove, Ian F Hermans and Gavin Frank Painter
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C4SC03599B, Edge Article
It is known that T cells can eliminate tumour cells through recognition of unique or aberrantly expressed antigens presented as peptide epitopes by major histocompatibility complex (MHC) molecules on the...
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC01737H, Edge Article
Site selectivity control is of vital importance in direct functionalization of inert C–H bonds. Reported here is a novel example of remote regiodivergent ortho- and meta-C–H bond functionalizations of phenylethylamine...
Dale C. Guenther, Grace H. Anderson, Saswata Karmakar, Brooke A. Anderson, Bradley A. Didion, Wei Guo, John P. Verstegen and Patrick J. Hrdlicka
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01238D, Edge Article
Optimized Invader probes enable efficient (C50 < 1 μM), fast (t50 < 3 h), kinetically stable (>24 h), and single nucleotide specific recognition of DNA targets.
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01251A, Edge Article
Tuning Ir d-orbital occupation via doping Cu into the IrO2 lattice to prepare a highly efficient oxygen evolution reaction catalyst, Cu0.3Ir0.7Oδ.
Xianjun Lang, Wei Hao, Wan Ru Leow, Shuzhou Li, Jincai Zhao and Xiaodong Chen
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC01813G, Edge Article
The selective aerobic oxidation of sulfides into sulfoxides on TiO2 under visible-light irradiation was accomplished through synergistic catalysis with triethylamine.
Haitang Shi, Meng Niu, Longfei Tan, Tianlong Liu, Haibo Shao, Changhui Fu, Xiangling Ren, Tengchuang Ma, Jun Ren, Linlin Li, Huiyu Liu, Ke Xu, Jianxin Wang, Fangqiong Tang and Xianwei Meng
Chem. Sci., 2015, Advance Article
DOI: 10.1039/C5SC00781J, Edge Article
This paper develops a simple multifunctional theranostic platform using an IL@ZrO2 nanostructure for CT imaging guided tumor microwave thermotherapy.
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC01436K, Edge Article
Cytosine methylation and hydroxymethylation are both important epigenetic modifications of DNA in mammalian cells. Therefore, profiling DNA (hydroxy)methylation across the genome is vital to understanding their roles in gene regulation....
Takahiro Sasamori, Tomohiro Sugahara, Tomohiro Agou, Koh Sugamata, Guo Jing-Dong, Shigeru Nagase and Norihiro Tokitoh
Chem. Sci., 2015, Accepted Manuscript
DOI: 10.1039/C5SC01266J, Edge Article
Reaction of the stable digermyne BbtGeGeBbt (Bbt = 2,6-[CH(SiMe3)2]2-4-[C(SiMe3)3]-C6H2) with ethylene initially afforded the corresponding 1,2-digermacyclobutene. Depending on the reaction conditions applied, further reaction of this 1,2-digermacyclobutene with ethylene furnished...

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