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Chemical Science

For findings of exceptional significance from across the chemical sciences
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Nengbo Zhu, Jianguo Zhao and Hongli Bao
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04274K, Edge Article
Iron-catalyzed methyl, ethyl and propyl Heck reactions were developed using readily available alkyl peroxides as alkyl sources.
 
Chao Chen, Zhegang Song, xiaoyan Zheng, Zikai He, Bin Liu, Xuhui Huang, Deling Kong, Dan Ding and Ben Zhong Tang
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC03859J, Edge Article
Photosensitizers are generally treated as key component for photodynamic therapy. Differently, we herein report an aggregation-induce emission luminogen (AIEgen)-based photosensitizer (TPE-Py-FFGYSA) that can serve as a non-toxic adjuvant to amplify...
 
Yeru Liang, Luyi Chen, Dongyang Zhuang, Hao Liu, Ruowen Fu, Mingqiu Zhang, Dingcai Wu and Krzysztof Matyjaszewski
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC03961H, Edge Article
Super-hierarchical carbons with a unique carbonaceous hybrid nanotube-interconnected porous network were fabricated by utilizing well-defined carbon nanotube@polystyrene bottlebrushes as building blocks.
 
Xiaowei Li, Xiangyang Yuan, Pengchi Deng, Lixi Chen, Yi Ren, Chengyuan Wang, Lixin Wu, Wen Feng, Bing Gong and Lihua Yuan
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04714A, Edge Article
The importance of macrocyclic shape-persistency in novel host–guest systems for the highly efficient template-directed synthesis of rotaxanes has been revealed.
 
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04465D, Edge Article
The synthesis of antimony-ligated dysprosium SMMs is described in addition to the unexpected reactivity of the SMMs in stibine dehydrocoupling catalysis.
 
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04354B, Edge Article
The formation of two-component molecular cocrystals can lead to the tunable excited state intramolecular proton transfer (ESIPT) process and emission, as first confirmed by both experimental and computational studies.
 
Verena Pfeifer, Travis Jones, Juan-Jesus Velesco-Velez, Rosa Arrigo, Simone Piccinin, Michael Haevecker, Axel Knop-Gericke and R Schlogl
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC04622C, Edge Article
Water splitting performed in acidic media relies on the exceptional performance of iridium-based materials to catalyze the oxygen evolution reaction (OER). In the present work, we use in situ X-ray...
 
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC04455G, Edge Article
Diarylamines are an important class of widely utilized chemicals, and development of diverse procedures for their synthesis is of great importance. Herein, we have successfully developed novel versatile catalytic procedures...
 
Jichen Dong, Huan Wang, Hailing Peng, Zhongfan Liu, Kaili Zhang and Feng Ding
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC04535A, Edge Article
The formation of grain boundaries (GBs) in a graphene film is both fundamentally interesting and practically important for many applications. A GB in graphene is known as a linear defect...
 
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04344E, Edge Article
We show that a QM-based predictor of a protein backbone and CB chemical shifts is of comparable accuracy to empirical chemical shift predictors after chemical shift-based structural refinement that removes small structural errors (errors in chemical shifts shown in red).
 
Sivan Lilienthal, Michael Klein, Ron Orbach, Itamar Willner , Francoise Remacle and Raphael Levine
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC03892A, Edge Article
Concentration of molecules can be changed by chemical reactions and thereby offer a continuous readout. Yet computer architecture is cast in textbooks in terms of binary valued, Boolean variables. To...
 
Maximillian T. W. Lee, Antoine Maruani, Daniel A. Richards, James R. Baker, Stephen Caddick and Vijay Chudasama
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC03655D, Edge Article
A novel reagent/strategy enables the controlled assembly of antibody conjugates with a loading of two modules without antibody engineering.
 
D. J. van Dijken, P. Štacko, M. C. A. Stuart, W. R. Browne and B. L. Feringa
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC02935C, Edge Article
We report the design, synthesis and study of nanotube-forming light-responsive amphiphiles, in which chirality can be used as a means to control the morphologies of self-assembled structures.
 
Lev A. Dykman and Nikolai G. Khlebtsov
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC03631G, Perspective
This review summarizes what is known about the application of gold nanoparticles as an antigen carrier and adjuvant in immunization for the preparation of antibodies in vivo and evaluating their potential for the development of effective vaccines.
 
Yuncong Chen, Weijie Zhang, Yuanjing Cai, Ryan T. K. Kwok, Yubing Hu, Jacky W. Y. Lam, Xinggui Gu, Zikai He, Zheng Zhao, Xiaoyan Zheng, Bin Chen, Chen Gui and Ben Zhong Tang
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04206F, Edge Article
A novel dark through-bond energy transfer (DTBET) strategy is proposed and applied as the design strategy to develop ratiometric Hg2+ sensors with high performance.
 
Sandra Kaabel, Jasper Adamson, Filip Topić, Anniina Kiesilä, Elina Kalenius, Mario Öeren, Mart Reimund, Elena Shmatova, Aivar Lookene, H J Reich, Kari Rissanen and Riina Aav
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC05058A, Edge Article
A novel eight-membered macrocycle of the hemicucurbit[n]uril family, the chiral (all­R)­cyclohexanohemicucurbit[8]uril (cycHC[8]) binds anions in purely protic solvent with remarkable selectivity. The cycHC[8] portals open and close to fully encapsulate...
 
Hua Li, Deliang Zhang, Mengna Gao, Lumei Huang, Longguang Tang, Zijing Li, Xiaoyuan Shawn Chen and Xianzhong Zhang
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC04071C, Edge Article
A novel Förster resonance energy transfer (FRET) fluorescence “off-on” system based on highly specific, sensitive and effective C-C bond cleavage of certain dihydropyridine derivatives was reported for real-time quantitative imaging...
 
Chunchang Zhao, Ben Shi, Xianfeng Gu and Qiang Fei
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC04703C, Edge Article
H2S as a key chemical mediator exerts vital role in diverse physiological and pathological processes. However, the in vivo tracking of endogenous H2S generation still remains difficult due to the...
 
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC03590F, Edge Article
The orthogonality between the Schiff base reaction and boronic acid dehydration reaction is explored during the on-surface synthesis process. By simultaneous activation the above two reactions in one-step and employing...
 
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC02672A, Edge Article
Quantum mechanical calculations at various levels of theory indicate that charges (both “+” and “−”) on organic polymers can be stabilized by radicals on nearby polymer chains.
 
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04866H, Edge Article
Herein, a highly convergent strategy is developed to synthesize heneicosasaccharyl arabinomannan for the first time.
 
Jong-Sik Moon, Won-Geun Kim, Dong-Myeong Shin, So-Young Lee, Chuntae Kim, Yujin Lee, Jiye Han, Kyujung Kim, So Young Yoo and Jin-Woo Oh
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC02021F, Edge Article
A bioinspired M-13 bacteriophage-based photonic nose was developed for differential cell recognition.
 
M. J. Corr, S. V. Sharma, C. Pubill-Ulldemolins, R. T. Bown, P. Poirot, D. R. M. Smith, C. Cartmell, A. Abou Fayad and R. J. M. Goss
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04423A, Edge Article
Aqueous Sonogashira cross-coupling of unprotected bromotryptophan, tripeptides and a new to nature natural product (accessed through biosynthetic manipulation) is reported.
 
Junjiao Deng, Yi You, Heri BUSTAMANTE, Veena Sahajwalla and Rakesh K. Joshi
Chem. Sci., 2016, Accepted Manuscript
DOI: 10.1039/C6SC03909J, Minireview
It is understood that nano-channels of graphene oxide membranes share a water flow mechanisms which is similar to the water flow inside carbon nanotubes pores. Water transport mechanisms proposed by...
 
Prabhat Gautam, Rahul Sharma, Rajneesh Misra, M. L. Keshtov, S. A. Kuklin and Ganesh D. Sharma
Chem. Sci., 2017, Advance Article
DOI: 10.1039/C6SC04461A, Edge Article
Donor–acceptor–acceptor (D–A–A) type 1,8-naphthalimide based small molecules SM1 and SM2 functionalized with tetracyanobutadiene (TCBD) and dicyanoquino-dimethane (DCNQ) modules, showing strong absorption in the visible and near-infrared (NIR) region are reported.
 

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148 citations
A reversible photo-induced instability has been found in mixed-halide photovoltaic perovskites that limits the open circuit voltage in solar cells.
DOI: 10.1039/C4SC03141E
Published: 04 Nov 2014
39 citations
Direct splitting of pure water into H2 and O2 in a stoichiometric molar ratio of 2 : 1 by conjugated polymers via a 4-electron pathway was established for the first time, as demonstrated here using a g-C3N4 polymer and redox co-catalysts of Pt and Co species.
DOI: 10.1039/C5SC04572J
Published: 27 Jan 2016
65 citations
The combination of quantum yield and luminescence quenching measurements provides a method to rapidly characterize the occurrence of chain processes in a variety of photoredox reactions.
DOI: 10.1039/C5SC02185E
Published: 07 Jul 2015

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