Journal cover: Chemical Science

Chemical Science

For findings of exceptional significance from across the chemical sciences – moving to Gold Open Access in 2015
Impact Factor 8.314 12 Issues per Year ALPSP Award for Best New Journal 2011
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Michael A. Mercadante, Christopher B. Kelly, Trevor A. Hamlin, Kayla R. Delle Chiaie, Michael D. Drago, Katherine K. Duffy, Megan T. Dumas, Diana C. Fager, Bryanna L. C. Glod, Katherine E. Hansen, Cameron R. Hill, Rebecca M. Leising, Catherine L. Lynes, Allyson E. MacInnis, Madeline R. McGohey, Stephanie A. Murray, Marc C. Piquette, Shaina L. Roy, Ryan M. Smith, Katherine R. Sullivan, Bao H. Truong, Kristina M. Vailonis, Vitaliy Gorbatyuk, Nicholas E. Leadbeater and Leon J. Tilley
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01732C, Edge Article
Placement of an electron-withdrawing trifluoromethyl group (–CF3) at a putative cationic centre enhances γ-silyl neighbouring-group participation (NGP) resulting in ring closure via 1,3-γ-silyl elimination.
Alberto A. R. Mota, Pedro H. P. R. Carvalho, Bruna C. Guido, Heibbe C. B. de Oliveira, Thereza A. Soares, José R. Corrêa and Brenno A. D. Neto
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01785D, Edge Article
A novel lipophilic fluorescent small-molecule 2,1,3-benzothiadiazole derivative (named here as BTD-AO) was applied as a live cell-imaging probe for cellular uptake and dynamics studies at low temperature (4 °C) with an impressive selectivity staining exclusively lipid droplets.
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC00565A, Edge Article
Porous Co3O4 atomically-thin sheets with a thickness of 0.43 nm exhibit a 50-times higher electrocatalytic oxygen evolution current.
Adam S. Chatterley, Christopher W. West, Vasilios G. Stavros and Jan R. R. Verlet
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01493F, Edge Article
Time-resolved photoelectron spectroscopy of deprotonated nucleotides provides new insights into their relaxation dynamics.
Ampofo Darko, Stephen Wallace, Olga Dmitrenko, Melodie M. Machovina, Ryan A. Mehl, Jason W. Chin and Joseph M. Fox
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01348D, Edge Article
Computation has guided the design of conformationally-strained dioxolane-fused trans-cyclooctene (d-TCO) derivatives that display excellent reactivity in the tetrazine ligation.
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01545B, Edge Article
A highly efficient synthesis of aromatic amino acids via palladium-catalyzed arylation of the methyl group of alanine at room temperature.
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01272K, Edge Article
An oxophilic magnesium salt in combination with a chiral N,N′-dioxide ligand switches the chemoselectivity of an ambident nitrosocarbonyl species to nitrogen for the highly enantioselective α-amination of β-ketoesters.
Xin Zhong, Yanchao Wang, Feng Peng, Hanyu Liu, Hui Wang and Yanming Ma
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01383B, Edge Article
Using a CALYPSO structure searching method, bare C6 rings have been stabilized in the bulk crystal phases of charge-transfer systems at high pressures.
Yasuhiro Yamashita, Yuki Saito, Takaki Imaizumi and Shū Kobayashi
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01332H, Edge Article
We describe the concept of a Lewis acid/metal amide hybrid as a novel catalyst in acid/base catalysis.
Weiguang Ma, Dongxue Han, Min Zhou, Hao Sun, Lingnan Wang, Xiandui Dong and Li Niu
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC00826J, Edge Article
Using utg-C3N4/TiO2, a photoelectrochemical platform was designed for the sensing of global antioxidant capacity, which presented a rapid response, and anti-fouling and colour-interference-proof properties.
Depeng Zhao, Martín Fañanás-Mastral, Mu-Chieh Chang, Edwin Otten and Ben L Feringa
Chem. Sci., 2014, Accepted Manuscript
DOI: 10.1039/C4SC01940G, Edge Article
Chiral N,O-heterocycles were synthesized in high yields and excellent enantioselectivity up to 97% ee via iridium-catalysed intramolecular allylic substitution with nucleophilic attack of the amide oxygen atom. The resulting benzoxazine...
Ruohan Li, Shuzhang Xiao, Yi Li, Qifei Lin, Ronghua Zhang, Jun Zhao, Changying Yang, Kun Zou, Dongsheng Li and Tao Yi
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01243G, Edge Article
We report a unique example of polymorphism-dependent and piezochromic fluorescence, based on 2-(anthracen-9-yl)-4,5-diphenyl-1H-imidazole.
Haidong Feng, Kun Zhang and Jin Wang
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC00831F, Edge Article
Transition state or Kramers' rate theory has been used to quantify the kinetic speed of many chemical, physical and biological equilibrium processes successfully.
Xiaolong Sun, Qingling Xu, Gyoungmi Kim, Stephen E. Flower, John P. Lowe, Juyoung Yoon, John S. Fossey, Xuhong Qian, Steven D. Bull and Tony D. James
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01417K, Edge Article
A water-soluble boronate-based fluorescent probe was evaluated for the detection of peroxynitrite (ONOO) in the presence of a monosaccharide.
J. Ruiz-Rodríguez, M. Miguel, S. Preciado, G. A. Acosta, J. Adan, A. Bidon-Chanal, F. J. Luque, F. Mitjans, R. Lavilla and F. Albericio
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC00572D, Edge Article
Polythiazole amino acids clasp linear peptides to generate cyclic derivatives, however, the resulting species are not merely stapled peptides but bear a complex heterocyclic moiety displaying its intrinsic set of interactions.
Chem. Sci., 2014, Accepted Manuscript
DOI: 10.1039/C4SC01437E, Edge Article
The activities of hundreds of single molecules of β-galactosidase were monitored in the presence of fluorogenic substrates and two strong binding inhibitors—D-galactal and N-p-bromobenzylamino-hydroxymethyl-cyclopentanetriol (NpBHC). The stochastic binding and release...
Bin Yan Zhao, Jianlei Shen, Shixing Chen, Dongfang Wang, Fan Li, Sanjay Mathur, Shiping Song and Chunhai Fan
Chem. Sci., 2014, Accepted Manuscript
DOI: 10.1039/C4SC01792G, Edge Article
Surface-enhanced Raman scattering (SERS) technique has recently been used to design novel nanoprobes called "SERS tags" which hold great promise for the fields of biosensing and nanomedicine. More recent advances...
Pengfei Xu, Ranbo Yu, Hao Ren, Lingbo Zong, Jun Chen and Xianran Xing
Chem. Sci., 2014, Accepted Manuscript
DOI: 10.1039/C4SC01882F, Edge Article
Multi-shell ceria hollow spheres (MSCHSs) with uniform size of ~300nm and controlled shell number up to quadruple were synthesized by using carbonaceous spheres as the template in a combined process...
Jiandong Pang, Feilong Jiang, Daqiang Yuan, Jun Zheng, Mingyan Wu, Guoliang Liu, Kongzhao Su and Maochun Hong
Chem. Sci., 2014, Accepted Manuscript
DOI: 10.1039/C4SC01973C, Edge Article
Hexagonal-prismatic cages are constructed by cubane-like Ni4(μ3-OH)4 clusters generated with in situ and clip-like organic ligands. The SO42- anions template the formation of the above cages via weak cooperative C-H•••O...
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01221F, Edge Article
An effective and simple organocatalytic strategy for the synthesis of isoquinoline alkaloids.
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01549E, Edge Article
Wavelength dependent electron and hole distribution and dynamics of nanorod heterostructures leads to competing photoreduction pathways with different charge separation and recombination rates and steady state photoreduction quantum efficiencies.
Andrea Brugnara, Filip Topić, Kari Rissanen, Aurélien de la Lande, Benoit Colasson and Olivia Reinaud
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01457J, Edge Article
CuII coordination combined with hydrophobic pocket hosting allows for strong and selective fluoride binding in water at near neutral pH.
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC01339E, Minireview
Robust and reusable heterogeneous organometal catalysts open a new avenue to green chemical synthesis in water.
Nathan L. Bill, Masatoshi Ishida, Yuki Kawashima, Kei Ohkubo, Young Mo Sung, Vincent M. Lynch, Jong Min Lim, Dongho Kim, Jonathan L. Sessler and Shunichi Fukuzumi
Chem. Sci., 2014, Advance Article
DOI: 10.1039/C4SC00803K, Edge Article
Photoinduced electron transfer in a porphyrin supramolecule occurs to produce an 83 ms CS state.
Chem. Sci., 2014, Accepted Manuscript
DOI: 10.1039/C4SC01646G, Edge Article
Two nitrogen atoms and a flexible carbon skeleton make N, N, N’, N’-tetramethylethylenediamine (TMEDA) an important model system to study the interplay of conformeric motions and charge delocalization. Ionization of...

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