Neodymium(III) complexation by amino-carbohydrates via a ligand-controlled hydrolysis mechanism

Tatiana G. Levitskaia; Yongsheng Chen; John L. Fulton; Sergei I. Sinkov

doi:10.1039/C1CC11871D

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Chemical Communications

Issue 28, 2011

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Neodymium(III) complexation by amino-carbohydrates via a ligand-controlled hydrolysis mechanism

Tatiana G. Levitskaia,*^a Yongsheng Chen,^a John L. Fulton^a and Sergei I. Sinkov^a

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Pacific Northwest National Laboratory, 902 Battelle Blvd, PO BOX 999, MSIN P7-25, Richland, WA, USA
E-mail: Tatiana.levitskaia@pnl.gov;
Fax: +1 509 375 5684 ;
Tel: +1 509 375 5646

Chem. Commun., 2011,47, 8160-8162

DOI: 10.1039/C1CC11871D
Received 01 Apr 2011, Accepted 12 May 2011
First published online 17 Jun 2011

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Chelation of Nd³⁺ by D-glucosamine (DGA) and chitosan was investigated in solution at near-physiological pH and ionic strength. This research demonstrates the first example of the lanthanide ion heteroleptic hydroxo-carbohydrate complex in solution. Amino-carbohydrates DGA and chitosan suppressed formation of polynuclear Nd³⁺ species at elevated pH.

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