A novel multicomponent condensation, leading to the rare (Z)-chloromethyleneketals and their sulfur analogues, has been discovered. The mechanism of this reaction has been studied in some detail and subsequent modifications were performed on the adducts, leading to unusual Umpolung transforms.
F. Schevenels and I. E. Markó, Chem. Commun., 2011, 47, 3287 DOI: 10.1039/C0CC05186A
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