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Issue 38, 2010
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One-pot asymmetric cyclocarbohydroxylation sequence for the enantioselective synthesis of functionalised cyclopentanes

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Abstract

A new method has been developed for the enantioselective synthesis of highly functionalised cyclopentanes bearing up to three stereogenic centres with very high stereoselectivity. This one-pot process combines an enantioselective organocatalytic Michael addition with a highly diastereoselective [3+2]-cycloaddition–fragmentation step.

Graphical abstract: One-pot asymmetric cyclocarbohydroxylation sequence for the enantioselective synthesis of functionalised cyclopentanes

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Publication details

The article was received on 17 Jun 2010, accepted on 26 Jul 2010 and first published on 27 Aug 2010


Article type: Communication
DOI: 10.1039/C0CC01940B
Citation: Chem. Commun., 2010,46, 7247-7249
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    One-pot asymmetric cyclocarbohydroxylation sequence for the enantioselective synthesis of functionalised cyclopentanes

    W. Raimondi, G. Lettieri, J. Dulcère, D. Bonne and J. Rodriguez, Chem. Commun., 2010, 46, 7247
    DOI: 10.1039/C0CC01940B

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