Crystal structures of C60N2(C2H4)2 and C60{N2(C2H4)2}2 show that addition occurs with elongation of the C–C bond at the 6:6 ring junction to which the two nitrogen atoms are bonded; electrochemical one-electron reduction potentials of these adducts are shifted by ca. 0.1 V to more negative values for each added group.
A. L. Balch, B. Cullison, W. R. Fawcett, A. S. Ginwalla, M. M. Olmstead and K. Winkler, J. Chem. Soc., Chem. Commun., 1995, 2287 DOI: 10.1039/C39950002287
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