Enhanced Carrier Transport of Monolayer MoSe2 through Interlayer Coupling with In Situ Grown Metal-Organic Frameworks

Abstract

Exceptional interlayer coupling of organic-inorganic vdWHs is paramount for enhancing electron mobility. Herein, we report a novel transfer-free method to fabricate MoSe2/Ni3(HITP)2 vdWHs. The MOF film promotes interfacial charge transfer, leading to a threefold increase in electron mobility. This work provides a platform for developing high-performance optoelectronic devices.