Issue 21, 2022

Reply to the ‘Comment on “Terahertz pump–probe of liquid water at 12.3 THz”’ by A. F. G. van der Meer, PCCP, 2022, 24, D1CP05216K

Abstract

As outlined in our paper, we developed a model which is able to explain all recorded THz pump–probe data at 12.3 THz in the static water cell as well as in the liquid jet. The model includes an instantaneous temperature-dependent response by an acoustic phonon, an inherent non-linear response of water, and a slower thermal response. The order of magnitude of the non-linear contributions agrees with previous experimental results by us2 and other groups (see ref. 32, 33 and 35 in ref. 1) as well as with simulations2, which predict an enhanced non-linear response of water in the frequency range of the libration.

Graphical abstract: Reply to the ‘Comment on “Terahertz pump–probe of liquid water at 12.3 THz”’ by A. F. G. van der Meer, PCCP, 2022, 24, D1CP05216K

Associated articles

Article information

Article type
Comment
Submitted
03 Feb 2022
Accepted
05 May 2022
First published
20 May 2022

Phys. Chem. Chem. Phys., 2022,24, 13413-13415

Reply to the ‘Comment on “Terahertz pump–probe of liquid water at 12.3 THz”’ by A. F. G. van der Meer, PCCP, 2022, 24, D1CP05216K

F. Novelli, C. Hoberg, E. M. Adams, J. M. Klopf and M. Havenith, Phys. Chem. Chem. Phys., 2022, 24, 13413 DOI: 10.1039/D2CP00565D

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