Synergistic catalysis of graphitic carbon nitride supported bimetallic sulfide nanostructures for efficient oxygen generation

Abstract

Herein, a series of g-C₃N₄ supported bimetallic sulfide nanostructures (Ni₃S₂/MoS₂/ng-C₃N₄, n = 10, 20 and 30) was prepared by a hydrothermal method and subsequently a thermal annealing approach. Ni₃S₂/MoS₂/20g-C₃N₄ with controlled composition exhibits efficient OER activity with a low overpotential of 183 mV at 10 mA cm⁻², which outperforms the vast majority of sulfide OER electrocatalysts reported previously.