Ethylene oligomerization on Ni2+ single sites within lacunary defects of Wells Dawson polyoxometalates

Yoonrae Cho; Jessica A. Muhlenkamp; Allen G. Oliver; Jason C. Hicks

doi:10.1039/D1CC05377A

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Ethylene oligomerization on Ni²⁺ single sites within lacunary defects of Wells Dawson polyoxometalates†

Yoonrae Cho,

^a Jessica A. Muhlenkamp,^a Allen G. Oliver^b and Jason C. Hicks

*^a

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* Corresponding authors

^a Department of Chemical and Biomolecular Engineering, University of Notre Dame, 250 Nieuwland Hall, Notre Dame, IN 46556
E-mail: jhicks3@nd.edu

^b Department of Chemistry and Biochemistry, University of Notre Dame, 251 Nieuwland Hall, Notre Dame, IN 46556

Abstract

Oligomerization of light olefins has become an essential step to convert gaseous olefins to liquid fuels and value-added chemicals. Here, we report the synthesis and application of nickel single sites isolated on Wells Dawson polyoxometalate defects as stable and regenerable catalysts for ethylene oligomerization.

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Article information

DOI: https://doi.org/10.1039/D1CC05377A
Article type: Communication
Submitted: 23 Sep 2021
Accepted: 30 Nov 2021
First published: 30 Nov 2021

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Chem. Commun., 2021,57, 13772-13775

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Ethylene oligomerization on Ni²⁺ single sites within lacunary defects of Wells Dawson polyoxometalates

Y. Cho, J. A. Muhlenkamp, A. G. Oliver and J. C. Hicks, Chem. Commun., 2021, 57, 13772 DOI: 10.1039/D1CC05377A

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