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The radical acylarylation of N-arylacrylamides with aliphatic aldehydes using the photolysis of hypervalent iodine(III) reagents

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Abstract

This article describes a variety of 3,3-disubstituted 2-oxindoles that bear carbonyl groups, which are efficiently obtained from a radical reaction between N-arylacrylamides and aliphatic aldehydes. The reaction is initiated by the photolysis of hypervalent iodine(III) reagents and proceeds smoothly under mild, metal-free conditions.

Graphical abstract: The radical acylarylation of N-arylacrylamides with aliphatic aldehydes using the photolysis of hypervalent iodine(iii) reagents

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Publication details

The article was received on 15 Jun 2018, accepted on 13 Jul 2018 and first published on 14 Jul 2018


Article type: Communication
DOI: 10.1039/C8OB01420E
Citation: Org. Biomol. Chem., 2018, Advance Article
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    The radical acylarylation of N-arylacrylamides with aliphatic aldehydes using the photolysis of hypervalent iodine(III) reagents

    R. Sakamoto, N. Hirama and K. Maruoka, Org. Biomol. Chem., 2018, Advance Article , DOI: 10.1039/C8OB01420E

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