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Hydrogen bond directed aerobic oxidation of amines via photoredox catalysis

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Abstract

An application of H-bonding interactions for directing the α-C–H oxidation of amines to amides and amino-ketones catalyzed by an organic photocatalyst is reported. The high efficiency of this method is demonstrated by the aerobic oxidation of pyrrolidines, diarylamines and benzylamines bearing urea groups with high yields and a wide substrate scope.

Graphical abstract: Hydrogen bond directed aerobic oxidation of amines via photoredox catalysis

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Publication details

The article was received on 13 Aug 2018, accepted on 04 Sep 2018 and first published on 04 Sep 2018


Article type: Communication
DOI: 10.1039/C8CC06603E
Citation: Chem. Commun., 2018, Advance Article
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    Hydrogen bond directed aerobic oxidation of amines via photoredox catalysis

    H. Wang, Y. Man, K. Wang, X. Wan, L. Tong, N. Li and B. Tang, Chem. Commun., 2018, Advance Article , DOI: 10.1039/C8CC06603E

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