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Nucleobases and their derivatives related two-dimensional self-assembled nanostructures on Au(111)

Abstract

The construction of two-dimensional (2D) self-assembled nanostructures has been one of the considerably interesting areas of on-surface chemistry in the past few decades, which is benefited from the rapid development and improvement of scanning probe microscopy techniques. In this research field, many attempts have been made to the controllable fabrication of well-ordered and multifunctional surface nanostructures, which attracted interest because of the prospect for artificial design of functional molecular nanodevices. DNA and RNA are considered to be programmable self-assembly systems and it is possible to use their base sequences to encode instructions for assembly in a predetermined fashion at the nanometer scale. As important constituents of nucleic acids, nucleobases, with intrinsic functional groups for hydrogen bonding, coordination bonding, and electrostatic interactions, can be employed as a potential system for the versatile construction of various biomolecular nanostructures, which may be used to structure the self-assembly of DNA-based artificial molecular constructions and play the important role in the novel biosensors based on surface functionalization. In this article, we will review the recent progresses of on-surface self-assembly of nucleobases and their derivatives together with different reactants (e.g., metals, halogens, salts and water), and as a result, various 2D surface nanostructures are summarized.

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Publication details

The article was received on 04 May 2018, accepted on 10 Jul 2018 and first published on 10 Jul 2018


Article type: Feature Article
DOI: 10.1039/C8CC03585G
Citation: Chem. Commun., 2018, Accepted Manuscript
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    Nucleobases and their derivatives related two-dimensional self-assembled nanostructures on Au(111)

    Y. Ding, X. Wang, L. Xie, X. Yao and W. Xu, Chem. Commun., 2018, Accepted Manuscript , DOI: 10.1039/C8CC03585G

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