Issue 69, 2016
From the journal:

Chemical Communications

A N-heterocyclic tetracarbene Pd(ii) moiety containing a Pd(ii)–Pb(ii) bimetallic MOF for three-component cyclotrimerization via benzyne†

Ying Dong,a   Yue Li,a   Yong-Liang Wei,a   Jian-Cheng Wang,a   Jian-Ping Ma,a   Jun Ji,a   Bing-Jian Yaoa  and  Yu-Bin Dong*a  

* Corresponding authors

a College of Chemistry, Chemical Engineering and Materials Science, Key Laboratory of Molecular and Nano Probes, Engineering Research Center of Pesticide and Medicine Intermediate Clean Production, Ministry of Education, Shandong Provincial Key Laboratory of Clean Production of Fine Chemicals, Shandong Normal University, Wenhua East Road, Jinan 250014, People's Republic of China
E-mail: yubindong@sdnu.edu.cn

Abstract

A novel Pd(II)–Pb(II) bimetallic metal–organic framework Pd(II)–Pb(II)–MOF (B) which contains an N-heterocyclic tetracarbene Pd(II) moiety was synthesized based on a chelating N-heterocyclic dicarbene Pd(II)–NHDC ligand (A) under solvothermal conditions. It can be a highly active heterogeneous catalyst for three-component cyclotrimerization via benzyne species.

Graphical abstract: A N-heterocyclic tetracarbene Pd(ii) moiety containing a Pd(ii)–Pb(ii) bimetallic MOF for three-component cyclotrimerization via benzyne

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Article information

DOI
https://doi.org/10.1039/C6CC04570G
Article type
Communication
Submitted
01 Jun 2016
Accepted
28 Jul 2016
First published
28 Jul 2016

Chem. Commun., 2016,52, 10505-10508

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A N-heterocyclic tetracarbene Pd(II) moiety containing a Pd(II)–Pb(II) bimetallic MOF for three-component cyclotrimerization via benzyne

Y. Dong, Y. Li, Y. Wei, J. Wang, J. Ma, J. Ji, B. Yao and Y. Dong, Chem. Commun., 2016, 52, 10505 DOI: 10.1039/C6CC04570G

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