A one-pot I2-mediated annulation reaction of substrates containing diamino groups and aldehydes has been developed via oxidative C–N bond formation. This general and environmentally benign synthetic approach provides facile access to a variety of 1,3-diazaheterocyclic compounds, including quinazolinones, benzimidazoles, and cyclic amidines.
The article was received on 13 Jun 2015, accepted on 14 Jul 2015 and first published on 14 Jul 2015
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