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Issue 20, 2014
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Total synthesis of lycorine-type alkaloids by cyclopropyl ring-opening rearrangement

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Abstract

A practical method for the synthesis of lycorine-type alkaloids with cis-B/C ring structure has been developed. Based on the reactions of aminocyclization, palladium-mediated arylation and especially cyclopropyl ring-opening rearrangement, the synthesis of anhydrocaranine, (±)-γ-lycorane and putative (±)-amarbellisine was accomplished.

Graphical abstract: Total synthesis of lycorine-type alkaloids by cyclopropyl ring-opening rearrangement

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Publication details

The article was received on 17 Jan 2014, accepted on 11 Mar 2014 and first published on 11 Mar 2014


Article type: Paper
DOI: 10.1039/C4OB00126E
Citation: Org. Biomol. Chem., 2014,12, 3191-3200
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    Total synthesis of lycorine-type alkaloids by cyclopropyl ring-opening rearrangement

    D. Liu, L. Ai, F. Li, A. Zhao, J. Chen, H. Zhang and J. Liu, Org. Biomol. Chem., 2014, 12, 3191
    DOI: 10.1039/C4OB00126E

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