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Issue 20, 2014
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Rh(III)-Catalyzed intramolecular redox-neutral cyclization of alkenes via C–H activation

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Abstract

Biologically interesting fused oligocyclic lactams have been prepared via an intramolecular redox-neutral cyclization process. By the proper choice of the substrates with a wide variety of tethered olefins, the less favored C–H bond can be activated and functionalized. This C–H activation proceeds under mild conditions, obviates the need for external oxidants, and displays a broad scope with respect to the substituents.

Graphical abstract: Rh(iii)-Catalyzed intramolecular redox-neutral cyclization of alkenes via C–H activation

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Publication details

The article was received on 02 Jan 2014, accepted on 14 Jan 2014 and first published on 15 Jan 2014


Article type: Communication
DOI: 10.1039/C4CC00029C
Citation: Chem. Commun., 2014,50, 2650-2652
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    Rh(III)-Catalyzed intramolecular redox-neutral cyclization of alkenes via C–H activation

    Z. Shi, M. Boultadakis-Arapinis, D. C. Koester and F. Glorius, Chem. Commun., 2014, 50, 2650
    DOI: 10.1039/C4CC00029C

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