Issue 7, 2014
From the journal:

Chemical Communications

A proton channel allows a hydrogen oxidation catalyst to operate at a moderate overpotential with water acting as a base†

Sheri Lense,a   Arnab Dutta,a   John A. S. Robertsa  and  Wendy J. Shaw*a  

* Corresponding authors

a Pacific Northwest National Laboratory, PO Box 999, Richland, WA 99352, USA
E-mail: wendy.shaw@pnnl.gov
Tel: +1 509-375-5922

Abstract

We report the incorporation of a simple enzyme-inspired proton channel onto a hydrogen oxidation catalyst. This modification facilitates proton transfer and lowers the overpotential for oxidation of H2 by 300 mV when using water as a base.

Graphical abstract: A proton channel allows a hydrogen oxidation catalyst to operate at a moderate overpotential with water acting as a base

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Article information

DOI
https://doi.org/10.1039/C3CC46829A
Article type
Communication
Submitted
06 Sep 2013
Accepted
23 Nov 2013
First published
26 Nov 2013

Chem. Commun., 2014,50, 792-795

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A proton channel allows a hydrogen oxidation catalyst to operate at a moderate overpotential with water acting as a base

S. Lense, A. Dutta, J. A. S. Roberts and W. J. Shaw, Chem. Commun., 2014, 50, 792 DOI: 10.1039/C3CC46829A

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