Development of a new cascade reaction for convergent synthesis of pyrazolo[1,5-a]quinoline derivatives under transition-metal-free conditions

Jun-ya Kato; Hiroshi Aoyama; Tsutomu Yokomatsu

doi:10.1039/C2OB27050A

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Organic & Biomolecular Chemistry

Issue 7, 2013

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Development of a new cascade reaction for convergent synthesis of pyrazolo[1,5-a]quinoline derivatives under transition-metal-free conditions

Jun-ya Kato,^a Hiroshi Aoyama^a and Tsutomu Yokomatsu*^a

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School of Pharmacy, Tokyo University of Pharmacy and Life Sciences, 1432-1 Horinouchi, Hachioji, Tokyo 192-0392, Japan
E-mail: yokomatu@toyaku.ac.jp ;
Fax: +81-42-676-3239 ;
Tel: +81-42-676-3239

Org. Biomol. Chem., 2013,11, 1171-1178

DOI: 10.1039/C2OB27050A
Received 20 Oct 2012, Accepted 10 Dec 2012
First published online 11 Dec 2012

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A novel method for the synthesis of pyrazolo[1,5-a]quinolines under the transition-metal-free conditions has been developed. This method involves a novel combination of aromatic nucleophilic substitution and Knoevenagel condensation reactions to give pyrazolo[1,5-a]quinolines.

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Development of a new cascade reaction for convergent synthesis of pyrazolo[1,5-a]quinoline derivatives under transition-metal-free conditions

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