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Issue 2, 2013
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Straightforward heterogeneous palladium catalyzed synthesis of aryl ethers and aryl amines via a solvent free aerobic and non-aerobic dehydrogenative arylation

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Abstract

Aryl ethers have been prepared from cyclohexanone derivatives and various alcohols in the presence of a catalytic amount of palladium on charcoal. The formation of an enol ether followed by an aerobic or non-aerobic dehydrogenation reaction, seem to be the key steps of this transformation. In addition, this new method was also adapted for the synthesis of arylamines.

Graphical abstract: Straightforward heterogeneous palladium catalyzed synthesis of aryl ethers and aryl amines via a solvent free aerobic and non-aerobic dehydrogenative arylation

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Publication details

The article was received on 25 Oct 2012, accepted on 16 Nov 2012 and first published on 19 Nov 2012


Article type: Communication
DOI: 10.1039/C2GC36776A
Citation: Green Chem., 2013,15, 347-352
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    Straightforward heterogeneous palladium catalyzed synthesis of aryl ethers and aryl amines via a solvent free aerobic and non-aerobic dehydrogenative arylation

    M. Sutter, N. Sotto, Y. Raoul, E. Métay and M. Lemaire, Green Chem., 2013, 15, 347
    DOI: 10.1039/C2GC36776A

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