Strong field control of predissociation dynamics

María E. Corrales; Garikoitz Balerdi; Vincent Loriot; Rebeca de Nalda; Luis Bañares

doi:10.1039/C2FD20143G

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Strong field control of predissociation dynamics

María E. Corrales,^a Garikoitz Balerdi,^a Vincent Loriot,^a^b Rebeca de Nalda^b and Luis Bañares*^a

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Departamento de Química Física, Facultad de Ciencias Químicas (Unidad Asociada CSIC), Universidad Complutense de Madrid, 28040 Madrid, Spain
E-mail: banares@quim.ucm.es ;
Fax: +34913944135 ;
Tel: +34913944228

Instituto de Química Física Rocasolano, CSIC, C/Serrano 116, 28004 Madrid, Spain

Faraday Discuss., 2013, Advance Article

DOI: 10.1039/C2FD20143G
Received 06 Dec 2012, Accepted 17 Dec 2012
First published online 21 Dec 2012

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Strong field control scenarios are investigated in the CH₃I predissociation dynamics at the origin of the second absorption B-band, in which state-selective electronic predissociation occurs through the crossing with a valence dissociative state. Dynamic Stark control (DSC) and pump–dump strategies are shown capable of altering both the predissociation lifetime and the product branching ratio

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María E. Corrales
Garikoitz Balerdi
Vincent Loriot
Rebeca de Nalda
Luis Bañares

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