Linear trinuclear Zn(II)–Ce(III)–Zn(II) complex which behaves as a single-molecule magnet

Shiori Hino; Moe Maeda; Kei Yamashita; Yumiko Kataoka; Motohiro Nakano; Tomoo Yamamura; Hiroyuki Nojiri; Maiko Kofu; Osamu Yamamuro; Takashi Kajiwara

doi:10.1039/C2DT32812G

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Dalton Transactions

Issue 8, 2013

The international journal for inorganic, organometallic and bioinorganic chemistry

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Linear trinuclear Zn(II)–Ce(III)–Zn(II) complex which behaves as a single-molecule magnet

Shiori Hino,^a Moe Maeda,^a Kei Yamashita,^a Yumiko Kataoka,^a Motohiro Nakano,^b Tomoo Yamamura,^c Hiroyuki Nojiri,^c Maiko Kofu,^d Osamu Yamamuro^d and Takashi Kajiwara*^a

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Faculty of Science, Nara Women's University, Nara, Japan
E-mail: kajiwara@cc.nara-wu.ac.jp ;
Tel: +81-742-20-3402

Graduate School of Engineering, Osaka University, Suita, Japan

Institute for Materials Research, Tohoku University, Aoba-ku, Sendai, Japan

Institute for Solid State Physics, University of Tokyo, Kashiwa, Japan

Dalton Trans., 2013,42, 2683-2686

DOI: 10.1039/C2DT32812G
Received 24 Nov 2012, Accepted 21 Dec 2012
First published online 03 Jan 2013

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Linear Zn(II)–Ce(III)–Zn(II) complex, which involves only one 4f electron as a spin source, behaves as an SMM. Easy-axis magnetic anisotropy for the ground ²F_5/2 state of Ce(III) was achieved by a uni-axial crystal field, which is formed with four phenoxo oxygens as axial donors with the other five oxygens as equatorial donors.

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Linear trinuclear Zn(II)–Ce(III)–Zn(II) complex which behaves as a single-molecule magnet

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