A luminescent single-molecule magnet: observation of magnetic anisotropy using emission as a probe

Kei Yamashita; Rie Miyazaki; Yumiko Kataoka; Takayuki Nakanishi; Yasuchika Hasegawa; Motohiro Nakano; Tomoo Yamamura; Takashi Kajiwara

doi:10.1039/C2DT32785F

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Dalton Transactions

Issue 6, 2013

The international journal for inorganic, organometallic and bioinorganic chemistry

Impact Factor 3.838 48 Issues per Year Indexed in MEDLINE

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A luminescent single-molecule magnet: observation of magnetic anisotropy using emission as a probe

Kei Yamashita,^a Rie Miyazaki,^a Yumiko Kataoka,^a Takayuki Nakanishi,^b Yasuchika Hasegawa,*^b Motohiro Nakano,^c Tomoo Yamamura^d and Takashi Kajiwara*^a

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Faculty of Science, Nara Women's University, Kita-uoya Nishi-machi, Nara 630-8506, Japan
E-mail: kajiwara@cc.nara-wu.ac.jp ;
Tel: +81-742-20-3402

Division of Materials Chemistry, Graduate School of Engineering, Hokkaido University, Kita-ku, Sapporo, Japan
E-mail: hasegaway@eng.hokudai.ac.jp

Graduate School of Engineering, Osaka University, Suita, Japan

Institute for Materials Research, Tohoku University, Aoba-ku, Sendai, Japan

Dalton Trans., 2013,42, 1987-1990

DOI: 10.1039/C2DT32785F
Received 21 Nov 2012, Accepted 12 Dec 2012
First published online 13 Dec 2012

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An assemblage of a Tb(III) ion and two mononuclear [Zn^II(L)] complexes as antenna chromophores (H₂L: Schiff base ligand) afforded a luminescent single-molecule magnet. The f–f emission spectrum had partially resolved fine structure which provides detailed information on the magnetic anisotropy of the ⁷F₆ ground multiplet of the Tb(III) ion.

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Kei Yamashita
Rie Miyazaki
Yumiko Kataoka
Takayuki Nakanishi
Yasuchika Hasegawa
Motohiro Nakano
Tomoo Yamamura
Takashi Kajiwara

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A luminescent single-molecule magnet: observation of magnetic anisotropy using emission as a probe

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