Self-assembly between dicarboxylate ions and binuclear europium complexes: moving to water—pH dependence and effects of buffers

Leila R. Hill; Thomas Just Sørensen; Octavia A. Blackburn; Asha Brown; Paul D. Beer; Stephen Faulkner

doi:10.1039/C2DT32009F

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Dalton Transactions

Issue 1, 2013

The international journal for inorganic, organometallic and bioinorganic chemistry

Impact Factor 3.838 48 Issues per Year Indexed in MEDLINE

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Self-assembly between dicarboxylate ions and binuclear europium complexes: moving to water—pH dependence and effects of buffers

Leila R. Hill,^a Thomas Just Sørensen,*^a^b Octavia A. Blackburn,^a Asha Brown,^a Paul D. Beer^a and Stephen Faulkner*^a

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Corresponding authors

Chemistry Research Laboratory, Mansfield Road, Oxford, UK
E-mail: Stephen.Faulkner@chem.ox.ac.uk ;
Tel: +44 (0)1865 285148

Department of Chemistry, University of Copenhagen, Universitetsparken 5, DK-2100 København Ø, Denmark
E-mail: TJS@chem.ku.dk ;
Fax: +45 35 32 02 14 ;
Tel: +45 35 32 02 13

Dalton Trans., 2013,42, 67-70

DOI: 10.1039/C2DT32009F
Received 31 Aug 2012, Accepted 08 Oct 2012
First published online 09 Oct 2012

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Binuclear lanthanide complexes consisting of two lanthanide binding domains in kinetically stable DO3A binding pockets linked by a 3-functionalized meta-xylyl bridge form stable 1:1 adducts with isophthalate and dinicotinate in water. The influence of buffer, pH and ligand structure on the binding of dinicotinate has been investigated.