Single-molecule magnet based on a C-type polyoxomolybdate with an S = 11 ground state: [Fe5CoMo22As2O85(H2O)]15−

Yanzhong Zhen; Bin Liu; Lili Li; Danjun Wang; Ying Ma; Huaiming Hu; Shengli Gao; Ganglin Xue

doi:10.1039/C2DT31331F

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Dalton Transactions

Issue 1, 2013

The international journal for inorganic, organometallic and bioinorganic chemistry

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Single-molecule magnet based on a C-type polyoxomolybdate with an S = 11 ground state: [Fe₅CoMo₂₂As₂O₈₅(H₂O)]¹⁵⁻

Yanzhong Zhen,^a^b Bin Liu,^a Lili Li,^a Danjun Wang,^a^b Ying Ma,^a Huaiming Hu,^a Shengli Gao^a and Ganglin Xue*^a

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Key Laboratory of Synthetic and Natural Functional Molecule Chemistry (Ministry of Education), Department of Chemistry, Northwest University, Xi'an, 710069, China
E-mail: xglin707@163.com

College of Chemistry & Chemical Engineering, Yan'an University, Shaanxi Key Laboratory of Chemical Reaction Engineering, Yan'an 716000, China

Dalton Trans., 2013,42, 58-62

DOI: 10.1039/C2DT31331F
Received 21 Jun 2012, Accepted 19 Oct 2012
First published online 22 Oct 2012

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Abstract
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A C-type polyoxomolybdate containing a mixed-transition metal cluster Fe₅Co has been prepared as an ammonium salt, (NH₄)₁₅[Fe₅CoMo₂₂As₂O₈₅(H₂O)]·15H₂O (1). Interestingly, the magnetism measurements show that the compound exhibits not only an overall ferromagnetic cluster with a large spin ground state of S = 11 but also the behavior of single-molecule magnets.

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Yanzhong Zhen
Bin Liu
Lili Li
Danjun Wang
Ying Ma
Huaiming Hu
Shengli Gao
Ganglin Xue

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Dalton Transactions

Single-molecule magnet based on a C-type polyoxomolybdate with an S = 11 ground state: [Fe₅CoMo₂₂As₂O₈₅(H₂O)]¹⁵⁻

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Single-molecule magnet based on a C-type polyoxomolybdate with an S = 11 ground state: [Fe5CoMo22As2O85(H2O)]15−

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Single-molecule magnet based on a C-type polyoxomolybdate with an S = 11 ground state: [Fe₅CoMo₂₂As₂O₈₅(H₂O)]¹⁵⁻