A new class of highly solvatochromic dicyano rhenate(I) diimine complexes – synthesis, photophysics and photocatalysis

Larry Tso-Lun Lo; Sze-Wing Lai; Shek-Man Yiu; Chi-Chiu Ko

doi:10.1039/C3CC39189B

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Chemical Communications

Issue 23, 2013

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A new class of highly solvatochromic dicyano rhenate(I) diimine complexes – synthesis, photophysics and photocatalysis

Larry Tso-Lun Lo,^a Sze-Wing Lai,^a Shek-Man Yiu^a and Chi-Chiu Ko*^a

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Department of Biology and Chemistry, City University of Hong Kong, Tat Chee Avenue, Hong Kong, China
E-mail: vinccko@cityu.edu.hk ;
Fax: +852-3442-0522 ;
Tel: +852-3442-6958

Chem. Commun., 2013,49, 2311-2313

DOI: 10.1039/C3CC39189B
Received 24 Dec 2012, Accepted 01 Feb 2013
First published online 01 Feb 2013

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A new class of dicarbonyl dicyano rhenate(I) diimine complexes, cis,trans-[Re(CO)₂(CN)₂(N–N)]⁻, with highly environmentally sensitive MLCT absorption and emission properties was synthesised and characterised. Preliminary experiments revealed that these complexes are active photocatalysts for CO₂ reduction.

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