New donor–π–acceptor sensitizers containing 5H-[1,2,5]thiadiazolo [3,4-f]isoindole-5,7(6H)-dione and 6H-pyrrolo[3,4-g]quinoxaline-6,8(7H)-dione units

Hairong Li; Teck Ming Koh; Anders Hagfeldt; Michael Grätzel; Subodh G. Mhaisalkar; Andrew C. Grimsdale

doi:10.1039/C3CC00060E

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Chemical Communications

Issue 24, 2013

Urgent high quality communications from across the chemical sciences.

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New donor–π–acceptor sensitizers containing 5H-[1,2,5]thiadiazolo [3,4-f]isoindole-5,7(6H)-dione and 6H-pyrrolo[3,4-g]quinoxaline-6,8(7H)-dione units

Hairong Li,^a Teck Ming Koh,^a^b Anders Hagfeldt,^c Michael Grätzel,^d Subodh G. Mhaisalkar*^a^b and Andrew C. Grimsdale*^a^b

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Energy Research Institute @ NTU (ERI@N), Nanyang Technological University, 50 Nanyang Drive, Singapore 637553
E-mail: subodh@ntu.edu.sg

School of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798
E-mail: ACGrimsdale@ntu.edu.sg

Department of Chemistry – Ångström, Uppsala University, Box 523, 75120 Uppsala, Sweden

Laboratory for Photonics and Interfaces, Institute of Chemical Sciences and Engineering, School of Basic Sciences, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland

Chem. Commun., 2013,49, 2409-2411

DOI: 10.1039/C3CC00060E
Received 04 Jan 2013, Accepted 28 Jan 2013
First published online 29 Jan 2013

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Two new D–π–A sensitizers (L101 and L102) incorporating 5H-[1,2,5]thiadiazolo [3,4-f]isoindole-5,7(6H)-dione and 6H-pyrrolo[3,4-g]quinoxaline-6,8(7H)-dione core structures were synthesized and tested in liquid dye-sensitized solar cells (DSCs). L102 achieved a promising power conversion efficiency (PCE) of 6.2% (AM 1.5, 100 mW cm⁻²).

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Hairong Li
Teck Ming Koh
Anders Hagfeldt
Michael Grätzel
Subodh G. Mhaisalkar
Andrew C. Grimsdale

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Chemical Communications

New donor–π–acceptor sensitizers containing 5H-[1,2,5]thiadiazolo [3,4-f]isoindole-5,7(6H)-dione and 6H-pyrrolo[3,4-g]quinoxaline-6,8(7H)-dione units

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Chemical Communications

New donor–π–acceptor sensitizers containing 5H-[1,2,5]thiadiazolo [3,4-f]isoindole-5,7(6H)-dione and 6H-pyrrolo[3,4-g]quinoxaline-6,8(7H)-dione units

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