Metallic zinc- assisted synthesis of Ti3+ self-doped TiO2 with tunable phase composition and visible-light photocatalytic activity

Zhaoke Zheng; Baibiao Huang; Xiaodong Meng; Junpeng Wang; Shaoying Wang; Zaizhu Lou; Zeyan Wang; Xiaoyan Qin; Xiaoyang Zhang; Ying Dai

doi:10.1039/C2CC37976G

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Metallic zinc- assisted synthesis of Ti³⁺ self-doped TiO₂ with tunable phase composition and visible-light photocatalytic activity

Zhaoke Zheng,^a Baibiao Huang,*^a Xiaodong Meng,^a Junpeng Wang,^a Shaoying Wang,^a Zaizhu Lou,^a Zeyan Wang,^a Xiaoyan Qin,^a Xiaoyang Zhang^a and Ying Dai^b

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Corresponding authors

State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China
E-mail: bbhuang@sdu.edu.cn ;
Tel: +86-531-8836-6324

School of Physics, Shandong University, Jinan 250100, China

Chem. Commun., 2013,49, 868-870

DOI: 10.1039/C2CC37976G
Received 04 Nov 2012, Accepted 20 Nov 2012
First published online 20 Nov 2012

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Stable Ti³⁺ self-doped TiO₂ with tunable phase composition and highly efficient visible-light photoactivity (ca. 32.7 times stronger than an undoped sample for ˙OH formation) was synthesized via a facile metallic zinc-assisted method. The surface Ti³⁺ species can be stabilized by Zn doping, and the photocatalytic selectivity can be regulated by the phase composition.

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Metallic zinc- assisted synthesis of Ti3+ self-doped TiO2 with tunable phase composition and visible-light photocatalytic activity

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Metallic zinc- assisted synthesis of Ti³⁺ self-doped TiO₂ with tunable phase composition and visible-light photocatalytic activity