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The Pt(II) complexes (1–3) bearing tetradentate ONCN ligands display high emission quantum yields (0.76–0.90) and good thermal stability (Td > 400 °C). Complex 3 is an excellent green phosphorescence dopant for OLEDs with excellent efficiency and low efficiency roll-off (ηL, ηExt(max) = 66.7 cd A−1, 18.2%; ηL, ηExt (1000 cd m−2) = 65.1 cd A−1, 17.7%).
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