Crystal structure and carrier transport properties of a new semiconducting 2D coordination polymer with a 3,5-dimethylpiperidine dithiocarbamate ligand

Takashi Okubo; Haruho Anma; Naoya Tanaka; Kento Himoto; Shu Seki; Akinori Saeki; Masahiko Maekawa; Takayoshi Kuroda-Sowa

doi:10.1039/C2CC37137E

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Chemical Communications

Issue 39, 2013

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Crystal structure and carrier transport properties of a new semiconducting 2D coordination polymer with a 3,5-dimethylpiperidine dithiocarbamate ligand

Takashi Okubo,*^a^b Haruho Anma,^a Naoya Tanaka,^a Kento Himoto,^a Shu Seki,^c Akinori Saeki,^c^b Masahiko Maekawa^a and Takayoshi Kuroda-Sowa^a

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Kinki University, 3-4-1 Kowakae, Higashi-Osaka-shi, Japan
E-mail: okubo_t@chem.kindai.ac.jp ;
Fax: +81-6-6723-2721 ;
Tel: +81-6-6730-5880 (ex. 4117)

PRESTO, Japan Science and Technology Agency (JST), Japan

Department of Applied Chemistry, Osaka University, 2-1 Yamadaoka, Suita, Japan

Chem. Commun., 2013,49, 4316-4318

DOI: 10.1039/C2CC37137E
Received 01 Oct 2012, Accepted 10 Dec 2012
First published online 19 Dec 2012

This article is part of themed collection: Emerging Investigators 2013

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Abstract
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A novel mixed-valence Cu(I)–Cu(II) coordination polymer with an infinite two-dimensional structure, [Cu₃ICuIIBr₃(3,5-Dmpip-dtc)₂]_n (3,5-Dmpip-dtc⁻ = 3,5-dimethylpiperidine dithiocarbamate), was prepared, and its structure was characterized by X-ray diffraction. It shows semiconducting behavior with a relatively small activation energy and high carrier mobility, which were investigated using impedance spectroscopy and flash photolysis time-resolved microwave conductivity measurements, respectively.

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Takashi Okubo
Haruho Anma
Naoya Tanaka
Kento Himoto
Shu Seki
Akinori Saeki
Masahiko Maekawa
Takayoshi Kuroda-Sowa

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Chemical Communications

Crystal structure and carrier transport properties of a new semiconducting 2D coordination polymer with a 3,5-dimethylpiperidine dithiocarbamate ligand

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Chemical Communications

Crystal structure and carrier transport properties of a new semiconducting 2D coordination polymer with a 3,5-dimethylpiperidine dithiocarbamate ligand

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