An aggregation-induced emission luminophore with multi-stimuli single- and two-photon fluorescence switching and large two-photon absorption cross section

Bingjia Xu; Mingyuan Xie; Jiajun He; Bin Xu; Zhenguo Chi; Wenjing Tian; Long Jiang; Fuli Zhao; Siwei Liu; Yi Zhang; Zhizhan Xu; Jiarui Xu

doi:10.1039/C2CC36806D

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Chemical Communications

Issue 3, 2013

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An aggregation-induced emission luminophore with multi-stimuli single- and two-photon fluorescence switching and large two-photon absorption cross section

Bingjia Xu,^a Mingyuan Xie,^b Jiajun He,^a Bin Xu,^c Zhenguo Chi,*^a Wenjing Tian,^c Long Jiang,^a Fuli Zhao,*^b Siwei Liu,^a Yi Zhang,^a Zhizhan Xu^d and Jiarui Xu^a

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PCFM Lab, DSAPM Lab, KLGHEI of Environment and Energy Chemistry, State Key Laboratory of Optoelectronic Materials and Technologies, School of Chemistry and Chemical Engineering, Sun Yat-sen University, Guangzhou 510275, P. R. China
E-mail: chizhg@mail.sysu.edu.cn ;
Fax: +86 20 84112222 ;
Tel: +86 20 84112712

School of Physics and Engineering, Sun Yat-sen University, Guangzhou 510275, P. R. China
E-mail: stszfl@mail.sysu.edu.cn

State Key Laboratory of Supramolecular Structure and Material, Jilin University, Changchun 130012, P. R. China

State Key Laboratory of High Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, P. R. China

Chem. Commun., 2013,49, 273-275

DOI: 10.1039/C2CC36806D
Received 18 Sep 2012, Accepted 09 Nov 2012
First published online 13 Nov 2012

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A novel aggregation- and crystallization-induced emission luminophore (ENPOMe) containing tetraphenylethene and acrylonitrile moieties with high fluorescence efficiency (Φ_F of up to 0.85) has been easily synthesized. ENPOMe has an exceptionally large two-photon absorption cross section (σ) of 5548 GM, and exhibits striking multi-stimuli-responsive single- and two-photon fluorescence switching with excellent reversibility in the solid state.

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