Issue 3, 2013
From the journal:

Chemical Communications

Direct methane oxidation over Pt-modified nitrogen-doped carbons†

Mario Soorholtz,a   Robin J. White,‡*b   Tobias Zimmermann,a   Maria-Magdalena Titirici,b   Markus Antonietti,b   Regina Palkovits*ac  and  Ferdi Schüth*a  

* Corresponding authors

a Max-Planck-Institut für Kohlenforschung, Kaiser-Wilhelm-Platz 1, 45470 Mülheim an der Ruhr, Germany
E-mail: schueth@mpi-muelheim.mpg.de
Fax: +49 208 306 2995
Tel: +49 208 306 2373

b Max Planck Institute of Colloids and Interfaces, Am Mühlenberg 1, 14476 Potsdam, Germany
E-mail: robin.white@mpikg.mpg.de
Fax: +49 331 567 9502
Tel: +49 331 567 9508

c RWTH Aachen, Worringerweg 1, 52074 Aachen, Germany
E-mail: palkovits@itmc.rwth-aachen.de
Fax: +49 241-80-22177
Tel: +49 241 80 26497

Abstract

Nitrogen-doped carbons derived from biomass precursors were modified with Pt2+ and successfully tested as solid catalysts in the direct oxidation of methane in fuming sulfuric acid. Remarkably, the catalytic performance was found to be substantially better than the Pt-modified Covalent Triazine Framework (CTF) system previously reported, although deactivation is more pronounced for the biomass derived catalyst supports.

Graphical abstract: Direct methane oxidation over Pt-modified nitrogen-doped carbons

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Article information

DOI
https://doi.org/10.1039/C2CC36232E
Article type
Communication
Submitted
28 Oct 2011
Accepted
12 Nov 2012
First published
22 Nov 2012

Chem. Commun., 2013,49, 240-242

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Direct methane oxidation over Pt-modified nitrogen-doped carbons

M. Soorholtz, R. J. White, T. Zimmermann, M. Titirici, M. Antonietti, R. Palkovits and F. Schüth, Chem. Commun., 2013, 49, 240 DOI: 10.1039/C2CC36232E

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