Preparation and study of an f,f,f′,f′′ covalently linked tetranuclear hetero-trimetallic complex – a europium, terbium, dysprosium triad

Thomas Just Sørensen; Manuel Tropiano; Octavia A. Blackburn; James A. Tilney; Alan M. Kenwright; Stephen Faulkner

doi:10.1039/C2CC35931F

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Chemical Communications

Issue 8, 2013

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Preparation and study of an f,f,f′,f′′ covalently linked tetranuclear hetero-trimetallic complex – a europium, terbium, dysprosium triad

Thomas Just Sørensen,*^a^b Manuel Tropiano,^a Octavia A. Blackburn,^a James A. Tilney,^a Alan M. Kenwright^c and Stephen Faulkner*^a

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Chemical Research Laboratory, Oxford University, 12 Mansfield Road, Oxford OX1 3TA, England
E-mail: Stephen.Faulkner@chem.ox.ac.uk ;
Tel: +44 (0)1865 285148

Nano-Science Center and Department of Chemistry, University of Copenhagen, Universitetsparken 5, DK-2100 København Ø, Denmark
E-mail: TJS@chem.ku.dk ;
Fax: +45 35320214 ;
Tel: +45 35320213

Department of Chemistry, University of Durham, South Road, Durham DH1 3LE, UK

Chem. Commun., 2013,49, 783-785

DOI: 10.1039/C2CC35931F
Received 16 Aug 2012, Accepted 06 Dec 2012
First published online 07 Dec 2012

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A heterotrimetallic tetranuclear lanthanide complex containing two dysprosium ions, a terbium ion and a europium ion has been prepared by coupling three kinetically stable complexes together using the Ugi reaction. The covalently linked trimetallic system exhibits luminescence from all the different lanthanide centres.

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Thomas Just Sørensen
Manuel Tropiano
Octavia A. Blackburn
James A. Tilney
Alan M. Kenwright
Stephen Faulkner

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Chemical Communications

Preparation and study of an f,f,f′,f′′ covalently linked tetranuclear hetero-trimetallic complex – a europium, terbium, dysprosium triad

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Preparation and study of an f,f,f′,f′′ covalently linked tetranuclear hetero-trimetallic complex – a europium, terbium, dysprosium triad

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