Morphologies of block copolymers composed of charged and neutral blocks

Xiaojun Wang; Monojoy Goswami; Rajeev Kumar; Bobby G. Sumpter; Jimmy Mays

doi:10.1039/C2SM07223H

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Soft Matter

Issue 11, 2012

Where physics meets chemistry meets biology for fundamental soft matter research.

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Morphologies of block copolymers composed of charged and neutral blocks

Xiaojun Wang,^a Monojoy Goswami,^b Rajeev Kumar,^c Bobby G. Sumpter*^b^d and Jimmy Mays*^a^d^e

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Department of Chemistry, University of Tennessee at Knoxville, Knoxville, USA
E-mail: jimmymays@utk.edu

Computer Science and Mathematics Division, Oak Ridge National Laboratory, Oak Ridge, USA
E-mail: sumpterbg@ornl.gov

National Center for Computational Sciences, Oak Ridge National Laboratory, Oak Ridge, USA

Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, USA

Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, USA

Soft Matter, 2012,8, 3036-3052

DOI: 10.1039/C2SM07223H
Received 20 Nov 2011, Accepted 23 Jan 2012
First published online 08 Feb 2012

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This article reviews current experimental observations and theoretical calculations devoted towards understanding micro-phase separation in charged block copolymer systems. We discuss bulk morphologies in melt and in solution, as well as some of the new emerging research directions. Overall, a comprehensive picture is beginning to emerge on the fundamental role of electrostatics in the micro-phase separation of charged block copolymers. This understanding provides exciting new insight that may be used to direct targeted structures that endow the materials with desired properties that can have tremendous potential in technological applications.

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Monojoy Goswami
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Bobby G. Sumpter
Jimmy Mays

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