A highly selective vanadium catalyst for benzylic C–H oxidation

Ji-Bao Xia; Kevin W. Cormier; Chuo Chen

doi:10.1039/C2SC20178J

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Chemical Science

Issue 7, 2012

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A highly selective vanadium catalyst for benzylic C–H oxidation

Ji-Bao Xia,^a Kevin W. Cormier^a and Chuo Chen*^a

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Division of Chemistry, Department of Biochemistry, The University of Texas Southwestern Medical Center, Dallas, USA
E-mail: Chuo.Chen@UTSouthwestern.edu ;
Fax: +1 214 6480320 ;
Tel: +1 214 6485048

Chem. Sci., 2012,3, 2240-2245

DOI: 10.1039/C2SC20178J
Received 10 Feb 2012, Accepted 13 Apr 2012
First published online 13 Apr 2012

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Vanadium complexes have been used extensively to catalyze olefin and alcohol oxidation. However, their application in C–H oxidation has not been well-studied. We report herein that commercially available Cp₂VCl₂ catalyzes benzylic C–H oxidation selectively and effectively, giving no aromatic oxidation products.

Abstract from Catalysts & Catalysed Reactions 2012

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